It's kind of a long explanation, and I'll post it more in depth in the Frankentranny thread, but I measured/calculated the spring constants (for both the 5R55E and A4LD) for the main regulator springs (the larger diameter ones) by measuring the free length (zero force) and partially compressed length with a certain weight (in my case it was 5.53lb). With thse spring constants, the only other thing needed was the diameters of the main valves, which turned out to be 0.398" for the A4 and .420" for the 5R.
So for the A4LD, I got a value of 47.7 psi/inch. This means that if I want to raise the pressure by 5 psi, I would insert a spacer with a thickness of 0.105" (47.7X.105=5). A 10 psi increase would be 0.210", etc...
For the 5R55E, I got a value of 71.3 psi/inch.
The other thing that is a limit to how much you can "safely" raise the pressure is how much the main spring can be compressed before it is fully compressed and doesn't allow the valve to open (vent) so that the pressure can still be regulated.
Here's a picture of the regulator valve assemblies (5R55E on top, A4LD on bottom):
So basically, I'm putting in a spacer that will preload the main regulator spring, so it has the same inner and outer diameters as the boost valve sleeve (a little smaller for each diameter to make installation easier). This leaves the boost the same, it just raises the baseline regulated pressure -> so if it normally had 60 psi at idle and an additional 20 psi of boost (to give a 80 psi reading) in a particular gear/engine speed, it would have 70 psi at idle and an additional 20 psi of boost (to give a 90 psi reading).